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The Lust For Life singer said the music she made with the Scouse rocker was better suited to his solo record.
Lana Del Rey has revealed she formed a band with Miles Kane last year, but they have already axed the group.
The 32-year-old singer teamed up with the rocker and some of his The Last Shadow Puppets bandmates for a new project in December, but soon decided the songs were more suited to the 31-year-old star's solo work.
Speaking Zane Lowe on Beats 1, she said: "I've done so much with Miles. I think at first me and Miles and some of the guys in The Last Shadow Puppets were working on a side project and had our own band.
"This was December through March. I didn't have a world tour planned and they didn't have anything either cos Alex [Turner] is working on his stuff, but, after listening to the songs, I felt like the songs were probably for Miles' solo stuff."
The period was no doubt around the time Del Rey went for a spot of of karaoke with the Last Shadow Puppets duo in February.
The Born To Die singer added: "Him and [The Last Shadow Puppets bassist] Zach Dawes are working on that."
Miles Kane has enlisted the help of Jamie T on his upcoming record, sharing a pic with the Tinfoil Boy back in April.